# sudo nano /etc/default/limine
# Place just below the previous KERNEL_CMDLINE[default]+="quiet splash"
KERNEL_CMDLINE[default]+="ttm.pages_limit=25165824"
Both ttm.pages_limit and ttm.page_pool_size seems to default to half of the RAM size, see: drivers/gpu/drm/ttm/ttm_device.c:88-100. So changing just one parameter won’t change the other one automatically.
You can calculate the number of pages somewhat like this (just replace 100 with # of GB):
python3 -c "print(100 * 1024**3 // 4096)"
Also, @roosmaa above mentioned amdgpu.gttsize. Don’t use it. It is deprecated, see: amdgpu — Module Parameters — gttsize. Unless you explicitly touch this deprecated parameter, ttm.* are the only thing you need to change.